The Ultimate Guide to Thermal Evaporation Coatings

Thermal evaporation coating is one of the most basic and widely used thin film preparation methods in physical vapor deposition (PVD). Since its birth in the early 20th century, it has played an irreplaceable role in many fields such as optics, electronics, materials science, aerospace, etc.

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Everything You Should Know About Thermal Evaporation Coating

Thermal evaporation coating is one of the classic and mature physical vapor deposition technologies. With its clear principles, simple equipment, and stable film quality, it has always maintained strong vitality in the past 100 years of development. This blog explains the thermal evaporation coating system, from core principles to practical applications, and provides a reference for research in related fields.

Thermal evaporation coating is to heat the material to the evaporation temperature through specific heating in a high vacuum environment, so that it changes from solid to gas. The evaporated atoms or molecules are ejected to the substrate surface in a linear motion in a vacuum, and condense and deposit on the substrate. The atoms or molecules of the coating material shuttle freely in the form of gas, and finally arrange in an orderly manner on the surface of the substrate to build a layer of film with specific functions and performance.

Compared with other coating technologies, evaporation coating has unique advantages and characteristics. Its equipment is relatively simple, the cost is relatively low, and it is competitive in large-scale production. Evaporation coating achieves a high deposition rate. In a high vacuum environment, the introduction of impurities is effectively avoided, thereby obtaining high-purity film.

What is thermal evaporation coating

Principle of Thermal Evaporation Coating

In thermal evaporation coating, the vacuum environment is like a pure stage, providing the necessary conditions for the orderly “performance” of atoms and molecules. When the system is in a high vacuum state, the number of gas molecules is extremely small, which greatly reduces the probability of the evaporated atoms or molecules colliding with other gas molecules during transmission.

Heating Mechanism

Heating is one of the core links of evaporation coating, which transfers heat to the coating material to gradually increase its temperature. When the temperature reaches the evaporation temperature of the coating material, the material molecules obtain enough energy, overcome the interaction force between molecules, and begin to change from solid to gas, which is evaporation. The transfer and efficiency of heat directly affect the rate and uniformity of evaporation. Taking resistance heating as an example, heat is generated when current passes through the resistance wire. Heat conduction transfers the heat to the coating material. If the temperature distribution of the resistance wire is uneven, it will cause uneven heating of the coating material, thereby affecting the uniformity of evaporation.

Evaporation Mechanism

Evaporation is not a simple material state transition, which involves a complex evaporation dynamic mechanism. According to the molecular motion theory, the evaporation rate of a substance is closely related to factors such as temperature and the vapor pressure of the substance. The higher the vapor pressure of the substance, the faster the evaporation rate. When the coating material is heated, after the molecules on its surface obtain energy, some of the molecules will have enough energy to overcome the surface energy, thereby leaving the material surface and entering the gas phase. As the temperature rises, the number of molecules with this energy increases, and the evaporation rate also accelerates. Evaporation is also affected by factors such as the surface state of the material and the surrounding gas environment. If there are impurities or defects on the surface of the material, it may affect the evaporation behavior of the molecules; and the pressure and composition of the surrounding gas environment will also have a certain impact on the evaporation rate.

Deposition and Film Formation

When the evaporated atoms or molecules enter the vacuum environment in the form of gas, they will move freely in the vacuum to form an atomic flow or a molecular flow. Once these atoms or molecules come into contact with the substrate surface, they will be adsorbed by the substrate surface to form a physical adsorption layer. As the number of adsorbed atoms continues to increase, when a certain critical concentration is reached, tiny crystal nuclei will form on the substrate surface. Once the crystal nuclei are formed, they will continue to adsorb the surrounding atoms and gradually grow. Adjacent crystal nuclei will also fuse with each other to eventually form a continuous film. In the growth of thin films, atomic deposition rate and surface diffusion rate have an important influence on the structure and properties of the film.

If the atomic deposition rate is too fast and the surface diffusion rate is slow, it may lead to more defects and pores in the film; on the contrary, if the surface diffusion rate is fast, the atoms can be fully diffused and arranged in an orderly manner, and a film with a dense structure and excellent performance can be obtained.

Types of Thermal Evaporation Coating

Laser evaporation coating uses a high-energy-density laser beam to irradiate the coating material, so that it quickly absorbs the laser energy and the temperature rises sharply, thereby achieving instant evaporation. Laser evaporation coating has an extremely high evaporation rate and evaporation efficiency, and completes the deposition of thin films in a short time.

Resistor evaporation coating refers to the process in which the current passes through the resistor material to generate heat, which is transferred to the coating material to reach the evaporation temperature, thereby achieving coating. It is suitable for metals and alloys with low melting points, such as aluminum, silver, and copper.

Electron beam evaporation coating uses an electron gun to generate a high-speed electron beam. The electron beam is accelerated under the action of the electric field and focused on the coating material through an electromagnetic lens. The atoms or molecules obtain enough energy to transform from solid to gas to achieve evaporation.

Thermal Evaporation Coating Materials

SymbolMelting Point °CDensityZ-ratioTemperature °C @ Vapor Pressure (Torr)Evaporation MethodCrucible LinerRemarks
Al6602.71.086778211010eBeam (Xlnt)TiB2-TiC, TiB2-BN,High deposition rates possible. Al wets IMCS
graphite, BN
AlSb10804.3eBeam (fair)TiB2-BN, BN, C, Al2O3Co-evaporation is the best approach
AlAs16003.7~1300eBeam (poor)TiB2-BN, BN, Al2O3Co-evaporation can work but typically done with MBE
AlBr3973.01~50eBeam (poor)graphite, WeBeam or thermal evaporation of anhydrous AlBr3 powder
Al4C314002.36~800eBeam (fair)graphite, WeBeam evaporation from powder, but CVD is a better approach
Al2%Cu6402.8eBeam (fair)TiB2-TiC, BNeBeam evaporation of Al-Cu alloys is possible, but sputter deposition is a better approach
AlF312573.07410490700eBeam (fair)graphite, Mo, WFilms tend to be porous, but smooth
sublimessublimes
AlN3.26~1750eBeam (fair)TiB2-TiC,Reactive evaporation of Al in N2 or ammonia partial pressure
sublimesgraphite, BN
Al2O320453.970.3361550eBeam (Xlnt)W, graphiteSwept beam with low deposition rates (< 3 Å/sec)
Al2%Si6402.61010eBeam (fair)TiB2-TiC, BNeBeam evaporation of Al-Si alloys is possible, but sputter deposition is a better approach
Sb6306.68279345425eBeam (fair)BN, graphite, Al2O3As the deposition rate is increased from 3-5 Å/s the grain size decreases and film coverage improves
sublimes
Sb2Te36196.5600eBeam (fair)graphite, BN, WBest results are achieved with powdered source material, relatively high deposition rates can be achieved
Sb2O36565.2 or 5.76~300eBeam (good)BN, Al2O3eBeam evaporation from powder or granules
sublimes
Sb2Se3611eBeam (fair)graphiteCan be co-evaporated with Se to overcome variable stoichiometric effects
Sb2S35504.64~200eBeam (good)Al2O3, Mo, TaFilms without substrate heating are amorphous, while polycrystalline films form on heated substrates
As8145.73107150210eBeam (poor)Al2O3, BeO,Sputter deposition is the preferred method for deposition of elemental arsenic
graphite
As2Se33604.75eBeam (poor)Al2O3, quartzDeposition efficiency increases with deposition rate
As2S33003.43~400eBeam (fair)Al2O3, quartz, MoThin films tend to be richer in As compared to the source material
As2Te3362eBeam (poor)Al2O3, quartzCVD is the preferred deposition technique for this material
Ba7103.78545627735eBeam (fair)W, Ta, MoReacts with ceramics. Ba evaporation pellets are often shipped with protective coatings which must be removed
BaCl29623.86~650eBeam (poor)W, MoSwept beam and slow power ramp to precondition and outgas the source material
BaF212804.83~700eBeam (fair)W, MoBetter consistency in refractive index is achieved via CVD
sublimes
BaO19235.72 or 5.32~1300eBeam (fair)Al2O3, quartzSwept beam and slow power ramp to precondition and outgas the source material
BaS22004.251100eBeam (poor)W, MoSputter deposition is the preferred deposition technique
BaTiO3Decomposes6DecomposeseBeam (poor)W, MoBaTiO3 will decompose as single source. Co-evaporate with Ti to maintain Ba/Ti ratio
Be12781.857108781000eBeam (Xlnt)graphiteVery high deposition rates are possible. Avoid Be powder sources due to toxicity
BeCl24401.9~150eBeam (poor)graphiteCVD is the preferred deposition technique for this material
BeF28001.99~200eBeam (fair)graphiteAvoid powder sources due to toxicity
sublimes
BeO25303.011900eBeam (fair)graphite, Al2O3Thin films can also be produced via reactive evaporation of Be with O2
Bi2719.8330410520eBeam (Xlnt)Al2O3, graphitePost deposition thermal annealing significantly enhances film properties. However, vapors are toxic
BiF37278.75~300eBeam (poor)graphiteSublimes at relatively low temperature, so reasonable vapor pressure can be achieved
sublimes
Bi2O38208.9~1400eBeam (poor)eBeam evaporation from Bi2O3 source is possible, but variations in thin film stoichiometry may occur
Bi2Se37107.66~650eBeam (fair)graphite, quartzSputter deposition is preferred, but
co-evaporation using Bi and Se sources is possible
Bi2Te35857.85~600eBeam (fair)graphite, quartzSputter deposition is preferred, but
co-evaporation using Bi and Te sources is possible
Bi2Ti2O7DecomposeseBeam (poor)graphite, quartzDecomposes when evaporated. Sputter deposition is preferred, but can be reactively co-evaporated in O2 partial pressure
Bi2S36857.39eBeam (poor)graphite, WCan be co-evaporated from Bi and S sources
B21002.360.389127815481797eBeam (Xlnt)graphite, WCan react with graphite and tungsten crucible liners. Requires high power to evaporate
sublimes
B4C23502.5250025802650eBeam (good)graphite, WIon assisted eBeam deposition with Ar can improve film adhesion
BN23002.2~1600eBeam (poor)graphite, WIon assisted eBeam deposition with N2 produces stoichiometric thin films, but sputter deposition is preferred
sublimes
B2O34601.82~1400eBeam (good)W, MoeBeam evaporation from bulk source material produces stoichiometric thin films
B2S33101.55800eBeam (poor)graphite
Cd3218.6464120180eBeam (fair)Al2O3, quartzDedicated system is recommended, since Cd can contaminate other purity sensitive depositions
CdSb4566.92
Cd3As27216.21eBeam (poor)quartzThin films can be produced by eBeam evaporation from bulk source material, but CVD is a preferred deposition method
CdBr25675.19~300
CdCl25704.05~400
CdF210705.64~500
CdI24005.3~250CdI2 films have been deposited by thermal evaporation on glass substrates using stoichiometric powders
CdO9006.95~530eBeam (poor)Al2O3, quartzCan be produced by reactive evaporation of Cd in partial pressure of O2 or reactive sputtering with O2
CdSe12645.81540eBeam (good)Al2O3, quartz, graphiteeBeam evaporation from bulk source material produces uniform films
CdSiO2~600Reports in the literature of deposition by CVD
CdS17504.82550eBeam (fair)Al2O3, quartz, graphiteSubstrate heating improves film adhesion. Deposition rates of 15 Å/sec are possible
sublimes
CdTe10986.2450eBeam (fair)Al2O3, quartz, graphiteHigh quality CdTe thin films on glass substrates at 100°C have been fabricated with eBeam deposition
Ca8421.56272357459eBeam (poor)Al2O3, quartzLow partial pressure of O2 in the vacuum chamber is required to avoid oxidizing the Ca
sublimes
CaF213603.18~1100eBeam (Xlnt)quartz, TaDeposition rate of 20 Å/sec are easily achieved with eBeam deposition.
Substrate heating improves film quality
CaO25803.35~1700eBeam (poor)ZrO2, graphiteForms volatile oxides with W and Mo
CaO-SiO215402.9eBeam (good)quartzPost deposition thermal annealing at 500°C improves film quality and adhesion
CaS2.181100eBeam (poor)ZrO2, graphiteDecomposition of CaS bulk source material can be overcome by co- evaporation with S
sublimes
CaTiO319754.1149016001690eBeam (poor)Sputter deposition is the preferred method
CaWO416206.06eBeam (good)W, ZrO2Substrate heating improves the crystallinity of the deposit
C1.8-2.30.22165718672137eBeam (Xlnt)graphite, WBetter film adhesion results from eBeam evaporation compared to vacuum arc deposition
sublimessublimes
Ce7958.2397011501380eBeam (good)Al2O3, BeO,Ce deposits readily oxidize when exposed to air
graphite
CeO226007.3189020002310eBeam (good)graphite, TaStoichiometric films are best achieved using reactive evaporation with O2.
sublimesSubstrate heating improves film quality
CeF314186.16~900eBeam (good)Mo, Ta, WCan be produced using bulk source material. Substrate heating from
150-300°C improves adhesion and film quality
Ce2O316926.87eBeam (fair)graphite, TaMixed CeO2-Ce2O3 films can be reduced to Ce2O3 by heating in UHV at 725°C
Cs281.87-162230eBeam (poor)quartz
CsBr6364.44~400
CsCl6463.97~500
CsF6843.59~500
CsOH2723.67~550
CsI6214.51~500eBeam (poor)quartz, PtStoichiometric CsI films are possible from bulk, source material, but good film coverage can be a challenge
Na5Al3F142.9~800eBeam (poor)Al2O3Stoichiometric chiolite films are difficult to fabricate with eBeam evaporation
Cr18907.20.3058379771157eBeam (good)W, graphiteFilms are very adherent. High deposition rates possible, but uniformity can be an issue
sublimes
CrB27606.17
CrBr28424.36550
Cr3C218906.68~2000eBeam (fair)WCan be fabricated by co-evaporation of Cr and C
CrCl28242.75550
Cr2O324355.21~2000eBeam (good)WStoichiometry can be maintained by reactive evaporation in O2
Cr3Si17106.51
Cr-SiOInfluenced by CompositioneBeam (good)WThe quality Cr-SiO cermet films fabricated with eBeam evaporation improves with annealing at 425° C
Co14958.98509901200eBeam (Xlnt)Al2O3, BeO,Pellets or powder both work well as source material
graphite
CoBr26784.91400
sublimes
CoCl27403.36472
sublimes
CoO19355.68eBeam (fair)CoO can be fabricated by reactive evaporation with O2, but sputter deposition is the preferred fabrication method
Cu10838.920.4377278571017eBeam (Xlnt)Al2O3, Mo Ta,Poor adhesion on most substrates. Use thin adhesion layer of Cr or Ti
graphite
CuCl4223.53~600eBeam (poor)quartzStoichiometric CuCl films have been produced from pellets and powder source material
Cu2O12356~600eBeam (good)graphite, Al2O3, TaThin films have been fabricated from stoichiometric Cu2O powder
sublimes
CuS11136.75~500
sublimes
Na3AlF610002.9102012601480eBeam (good)W, graphiteGood films can be fabricated using pellets or powder source material.
Dy14098.54625750900eBeam (good)WQuality thin films can be fabricated from bulk source material
DyF313606~800eBeam (good)W, TaBulk source material is available in pellets and powder form
sublimes
Dy2O323407.81~1400eBeam (fair)WThin films have been fabricated from bulk source material
Er14979.060.74650775930eBeam (good)W, Ta
sublimes
ErF213806.5~950
Er2O324008.64~1600eBeam (fair)WReactive evaporation of bulk material in O2 atmosphere maintains stoichiometry.
Eu8225.26280360480eBeam (fair)Al2O3
sublimes
EuF213806.5~950
Eu2O324008.64~1600eBeam (good)WReactive evaporation of Eu2O3 powder or granules in O2 atmosphere maintains stoichiometry.
EuS5.75eBeam (good)WeBeam evaporation of EuS powder in UHV (10-8 torr base vacuum) has been reported in the literature
Gd13127.897609001175eBeam (Xlnt)Al203, WeBeam evaporation of Gd directly from the water cooled Cu hearth has been reported
Gd2O323107.41eBeam (fair)Al203, WReactive evaporation of Gd2O3 pellets in O2 maintains thin film stoichiometry. Refractive index increases with substrate heating
Ga305.9619742907eBeam (good)graphite, Al2O3, BeO, quartzAlloys with refractory metals
GaSb7105.6eBeam (fair)W, TaeBeam evaporation from bulk source material is possible
GaAs12385.3eBeam (good)graphite, WFilm quality is improved with ion assisted evaporation
GaN6.1~200eBeam (fair)graphite, Al2O3, BeO, quartzReactive evaporation of Ga in 10-3 N
sublimes2
Ga2O319005.88eBeam (fair)graphite, WReactive evaporation of Ga2O3 in O2 partial pressure maintains stoichiometry
GaP15404.1770920eBeam (fair)quartz, WCo-evaporation of Ga and P has been reported
Ge9375.350.5168129571167eBeam (Xlnt)Al2O3, quartz, graphite, NiUniform films achieved with slow power ramp and swept beam
Ge3N24505.2~650eBeam (poor)Sputtering is the preferred method of fabrication
sublimes
GeO210866.24~625eBeam (good)graphite, Al2O3, quartzGeO2 stoichiometry can be maintained by reactive evaporation of bulk source material in O2
GeTe7256.2381
Au106219.320.3818079471132eBeam (Xlnt)W, Al2O3,Metal spitting can be an issue. Mitigate by slow power ramp with swept beam and low carbon content in source material
graphite, BN
Hf223013.09216022503090eBeam (good)W
HfB2325010.5Fabrication of HfB2 films by CVD has been reported
HfC416012.2~2600
sublimes
HfN285213.8HfN films have been produced by reactive RF sputtering of Hf in N2 + Ar
HfO228129.68~2500eBeam (fair)graphite, WCan be fabricated by reactive evaporation in O2 or using bulk source material. Post process annealing at 500°C improves film quality
HfSi217507.2eBeam (fair)WHfSi2 thin films have been fabricated by eBeam evaporation of Hf on Si substrates followed by annealing at 750°C for an hour
Ho14708.8650770950eBeam (good)W
sublimes
HoF311437.64~800quartz
Ho2O323708.41eBeam (fair)WHo2O3 thin films have been fabricated by eBeam evaporation of powdered source material or reactive evaporation of Ho in O2
In1577.30.841487597742eBeam (Xlnt)Mo, graphite, Al2O3Wets Cu and W. Mo liner is preferred
InSb5355.8500~400eBeam (fair)graphite, WThin films fabricated using powdered source material
InAs9435.7780870970Sputter deposition is the preferred thin film fabrication technique
In2O315657.18~1200eBeam (good)Al2O3Thin films have been produced by reactive evaporation of powdered In2O3 in O2 partial pressure.
sublimes
InP10584.8630730eBeam (fair)graphite, WDeposits are P rich
In2Se38905.7eBeam (fair)graphite, WThin films have been fabricated by eBeam evaporation from powdered InSe. Post process annealing improves crystallinity
In2S310504,9850
sublimes
In2S6535.87650
In2Te36675.8Thin films from co-evaporation of In and Te sources has been reported.
In2O3– SnO218006.43-7.14eBeam (good)graphiteThin films have been produced from 90% In2O3-10%SnO2 powder in O2 partial pressure. Substrate temperature of 250°C improves electrical conductivity of resulting films
Ir245922.65185020802380eBeam (fair)WBetter uniformity and adhesion can be achieved using sputter deposition
Fe15357.860.3498589981180eBeam (Xlnt)Al2O3, BeO,Molten Fe will attack and adhere to graphite, severely limiting crucible liner life
graphite
FeBr26894.64561
FeCl26702.98300
sublimes
FeI25925.31400
FeO14255.7eBeam (poor)Sputter deposition preferred.
Fe2O315655.24eBeam (good)Al2O3, BeO,Fe2O3 thin films fabricated by reactive evaporation of Fe in 0.1 Pa O2 partial pressure has been reported
graphite
FeS11954.84
La9206.1799012121388eBeam (Xlnt)W, Ta
LaB622102.61eBeam (fair)LaB6 films and coatings are more commonly produced with sputter deposition.
LaBr37835.06
LaF314906900eBeam (good)Ta, MoIon assisted eBeam evaporation improves film density and adhesion
sublimes
La2O322505.841400eBeam (good)W, graphiteC contamination can occur with graphite crucible liners
Pb32811.341.13342427497eBeam (Xlnt)Al2O3, quartz, graphite, W
PbBr23736.66~300
PbCl25015.85~325
PbF28228.24~400
sublimes
PbI25026.16~500
PbO8909.53~550eBeam (fair)Al2O3, quartz, WStoichiometric PbO thin films can be produced using powdered source material
PbSnO311158.1670780905eBeam (poor)Al2O3, WDisproportionates
PbSe10658.1~500eBeam (fair)Al2O3, graphite
sublimes
PbS11147.5550eBeam (fair)Al2O3, quartzPost deposition annealing at 150°C improves the crystallinity of the films
sublimes
PbTe9178.167809101050eBeam (poor)Al2O3, graphiteFilms produced from bulk PbTe tend to be Te rich. Sputter deposition is preferred
PbTiO37.52eBeam (fair)W, TaThin films of PbTiO3 with reactive co- evaporation of PbO powder and TiO2 pellets in O2 partial pressure has been reported
Li1790.53227307407eBeam (good)Ta, Al2O3, BeOLi films oxidize readily in air
LiBr5473.46~500
LiCl6132.07400
LiF8702.687510201180eBeam (good)W, Mo, Ta, Al2O3Rate control important for optical films. Outgas prior to deposition rastered beam
LiI4464.06400
Li2O14272.01850
Lu16529.841300eBeam (Xlnt)Al2O3
Lu2O324899.811400eBeam (fair)Al2O3eBeam evaporation of powdered source material results in stoichiometric films by post deposition rapid thermal anneal in O2 at 400-600°C
Mg6511.74185247327eBeam (good)W, graphite, Al2O3Powder is flammable. High deposition rates are possible
sublimes
MgAl2O421353.6eBeam deposition from MgAl2O4 powder has been reported
MgBr27003.72~450
MgCl27082.32400
MgF212662.9-3.21000eBeam (Xlnt)Al2O3, graphite, MoBest optical properties result from substrate heating at 300°C and a deposition rate of ≤ 5 Å/sec
MgI27004.24200
MgO28003.581300eBeam (good)Al2O3, graphiteStoichiometric films result from reactive evaporation in partial pressure of 10-3 torr O2
Mn12447.2507572647eBeam (good)W, Al2O3, BeO
sublimes
MnBr26954.38500
MnCl26502.98450
MnO25355.03eBeam (poor)W, Mo, Al2O3Stoichiometric thin films have been produced by reactive evaporation of Mn powder in 10-3 torr O
2
MnS16153.991300
Hg-3913.55-68-42-6Toxic, not recommended for evaporation processes
HgS 8.1250eBeam (poor)Al2O3Toxic and decomposes, not recommended for evaporation processes
sublimessublimes
Mo261010.22159218222117eBeam (Xlnt)graphite, WFilms are smooth, hard and adherent
MoB221007.12
Mo2C26879.18Thin films of Mo2C by sputter deposition and CVD have been reported
MoS211854.8~50Fabrication of MoS2 by CVD has been reported
MoSi220506.3~50MoSi2 films have been produced by sputter deposition
MoO37954.7~900eBeam (fair)Al2O3, graphite, BN, MoSubstrate heating improves film crystallinity
Nd102477318711062eBeam (Xlnt)Al2O3, Ta
NdF314106.5~900eBeam (good)W, Mo, Al2O3Substrate heating at 360°C improved film quality
Nd2O322727.24~1400eBeam (good)W, TaFilms may be oxygen deficient. Refractive index increases with increasing substrate temperature
Ni14538.910.33192710721262eBeam (Xlnt)Al2O3, BeO, W,Differential thermal expansion between Ni and graphite can cause graphite crucible liners to crack on cooling
graphite
NiBr29634.64362
sublimes
NiCl210013.55444
sublimes
NiO19907.45~1470eBeam (good)Al2O3, WSubstrate temperature of 125°C improves film adhesion and quality. Use of NiO powder as source material mitigates spitting
Nb (Cb)24688.55172819772287eBeam (Xlnt)graphiteIon assisted eBeam evaporation modifies Nb film stress from tensile to compressive at a substrate temperature of 400°C
NbB230506.97
NbC38007.82eBeam (fair)graphiteNbC thin films on Ti has been reported
NbN25738.4eBeam (fair)graphite, WNbN films have been fabricated using reactive evaporation and reactive sputtering in N2. NbN films by ion assisted evaporation have also been reported
NbO6.271100
Nb2O515304.47Nb2O5 films produced by RF magnetron sputtering using a stoichiometric target have been reported
NbTe7.6
Nb3SneBeam (Xlnt)graphite, TaFilms produced by co-evaporation of Nb and Sn have been reported. Substrate heating improves film homogeneity
Nb2O317807.5
Os170022.5217024302760
Pd155012.41192eBeam (Xlnt)W, Al2O3,Susceptible to metal spitting. Mitigate with slow power ramp and longer soak before deposition
graphite
PdO8708.31575eBeam (poor)Al2O3Decomposes
P41.41.82327361402eBeam (poor)Al2O3Reacts violently in air
Pt176921.450.245129214921747eBeam (Xlnt)W, Al2O3,Low deposition rates (< 5 Å/sec) preferred for film uniformity. Carbon contamination with graphite liners is possible at high power
graphite
Pu63519Toxic. Radioactive
Po2549.4117170244Toxic. Radioactive
K640.862360125quartzHighly reactive in air
KBr7302.75~450quartzUse gentle preheat to outgas
KCl7761.98~510eBeam (fair)Ta, quartz, MoUse gentle preheat to outgas
KF8802.48~500eBeam (poor)quartzUse gentle preheat to outgas
KOH3602.04~400
KI723.13~500
Pr9316.788009501150eBeam (good)W, graphite, TaPr films will oxidize in air
Pr2O321256.881400eBeam (good)W, graphite, ThO2Loses oxygen. Reports of Pr2O3 thin films grown by MBE
10月8日10月6日10月4日
Ra7005246320416
Re318020.53192822072571eBeam (good)W, graphiteSubstrate heating at 600°C improves film properties
ReO32978.2~100eBeam (good)W, graphiteFilms produced by reactive evaporation of Re in 10-3 torr O
2
Rh196612.41127714721707eBeam (good)W, graphite
Rb38.51.47-337111quartz
RbCl7152.76~500quartz
RbI6423.55~400quartz
Ru270012.45178019902260eBeam (poor)WMaterial spits using eBeam. Sputter deposition is preferred
Sm10727.54373460573eBeam (good)Al2O3
Sm2O323507.43eBeam (good)WLoses oxygen. Sputter deposition is preferred
Sm2S319005.72
Sc15392.997148371002eBeam (Xlnt)W, Mo, Al2O3Alloys with Ta
Sc2O323003.86~400eBeam (fair)WLoses oxygen. Films produced by reactive sputtering in O2 have been reported
Se2174.7989125170eBeam (good)W, Mo, graphite, Al2O3Toxic. Can contaminate vacuum systems
Si14102.420.71299211471337eBeam (fair)Ta, graphite, BeOHigh deposition rates possible. Molten Si can attack graphite liners limiting crucible liner life
SiB62.47
SiC27003.221000eBeam (fair)WSputter deposition is the preferred thin film fabrication technique
SiO21610-17102.2-2.71~1025eBeam (Xlnt)Al2O3, Ta,Swept beam is critical to avoid hole drilling, since the source material will have a shallow melt pool
Influenced by compositiongraphite, W
SiO17022.1850eBeam (fair)W, Ta, graphiteThin films from bulk SiO material has been reported
sublimes
Si3N43.44~800Thin films of Si3N3 by reactive sputter deposition have been reported
sublimes
SiSe550
SiS1.85450
sublimes
SiTe24.39550
Ag96110.490.5298479581105eBeam (Xlnt)W, Al2O3, Ta,Swept beam during melt and focused beam during deposition is recommended for higher deposition rates
Mo, graphite
AgBr4326.47~380
AgCl4555.56~520
AgI5585.67~500Thin films of AgI fabricated by thermal evaporation have been reported
Na970.9774124192quartzUse gentle preheat to outgas. Metal reacts violently in air
NaBr7553.2~400
NaCl8012.16530Thin films of NaCl fabricated by thermal evaporation in Knudsen cells with quartz crucibles have been reported
NaCN563~550
NaF9882.79~700eBeam (good)W, Ta, graphite, BeOUse gentle preheat to outgas. NaF thin films produced from powder source material and 230°C substrate heating have been reported
NaOH3182.13~470
Sr7692.6239309403eBeam (poor)graphite, quartzWets refractory metals. May react strongly in air
SrF211904.24~1000eBeam (poor)Al2O3, W, quartzThin films of SrF2 produced by eBeam and thermal evaporation have been reported
SrO24604.71500eBeam (poor)Al2O3Loses oxygen. Reacts with W and Mo
sublimes
SrS>20003.7Decomposes
S81152131957eBeam (poor)quartzCan contaminate vacuum systems
Ta299616.6196022402590eBeam (Xlnt)graphiteHigh melting point of Ta limits crucible liner selection. High vacuum is required to mitigate oxygen incorporation in films
TaB2300012.38
TaC388014.65~2500
TaN336016.3eBeam (fair)graphiteThin films of TaN can be produced by reactive evaporation in 10-3 torr N
2
Ta2O518008.74155017801920eBeam (good)graphite, TaSwept beam to avoid hole drilling. A thin Ti layer will improve adhesion to the substrate
TaS21300
Tc220011.5157018002090
Te4526.25157207277eBeam (poor)Al2O3, quartz, graphiteWets refractory metals
Tb13578.278009501150eBeam (Xlnt)Al2O3, graphite, TaThin films produced by sputter deposition and thermal evaporation have also been reported
TbF31176~800Sputter deposition is preferred
Tb2O323877.871300Thin films prepared by pulsed laser deposition have been reported
Tb4O723407.3Annealing of Tb2O3 films at 800°C in air to produce stable Tb4O7 has been reported
Tl30211.85280360470eBeam (poor)Al2O3, quartz, graphiteThallium and its compounds are very toxic. Wets freely
Tlbr4807.56~250Thermal evaporation of TlBr thin films has been reported
sublimes
TlCl4307~150
sublimes
TlI4407.09~250eBeam (poor)Al2O3, quartzLow stress thin films can be produced by eBeam evaporation with a substrate temperature of 100°C
 
Tl2O37179.65350Disproportionates at 850°C to Tl2O
Th187511.7143016601925eBeam (Xlnt)W, Ta, MoToxic and mildly radioactive
ThBr45.67
sublimes
ThC222738.96~2300
ThO2305010.03~2100eBeam (good)WStable stoichiometric films of ThO2 produced from powdered source material have been reported
ThF411106.3~750eBeam (fair)Ta, Mo, graphiteUse gentle preheat to outgas. Substrate temperature of 175°C improves film adhesion and quality
ThOF29009.1eBeam (poor)W, Ta, Mo,Does not evaporate stoichiometrically, resulting films are primarily ThF4
graphite
ThS26.8
Tm15459.32461554680eBeam (good)Al2O3
sublimes
Tm2O38.91500Thin films of Tm2O3 by eBeam evaporation and MBE have been reported
Sn2327.750.724682807997eBeam (Xlnt)Al2O3, Ta,High deposition rates possible, but uniformity may suffer. Slow power ramp to mitigate cavitation of melt pool
graphite, W
SnO211276.95~1000eBeam (Xlnt)Al2O3, quartzSubstrate temperature above 200°C improves film crystallinity
sublimes
SnSe8616.18~400Stoichiometric thin films of SnSe produced by thermal evaporation of powdered source material have been reported
SnS8825.08~450eBeam (poor)quartz, WThin films prepared by eBeam evaporation of SnS powder and reactive co-evaporation of Sn and S have been reported
SnTe7806.44~450eBeam (poor)quartzThin films of SnTe produced with eBeam evaporation at a substrate temperature of 300°C have been reported
Ti16754.50.628106712351453eBeam (Xlnt)W, graphite, TiCFilms are very adherent to almost any substrate
TiB229804.5Sputter deposition is the preferred thin film fabrication technique
TiC31404.93~2300eBeam (fair)W, graphiteeBeam evaporation of TiC thin films with and without ion beam assistance have been reported
TiO216404.29~1300eBeam (good)W, graphite, TaStoichiometric thin films of TiO2 have been produced from powder source material and a substrate temperature of 600°C
TiO1750~1500eBeam (good)W, graphite, TaOutgas with gentle preheat prior to deposition
TiN29305.43eBeam (good)W, graphite, TiCThin films have been prepared by reactive evaporation of Ti in N2 partial pressure
Ti2O321304.6eBeam (good)W, Ta, graphiteStoichiometric films have been produced by reactive evaporation of Ti O powder in 2.5 x 10-4 torr O
2 3 2
W341019.30.163211724072757eBeam (good)WLong, slow preheat is required to condition the source material. Raster the electron beam to avoid hole drilling
WB2290012.75
W2C286017.15148017202120eBeam (good)W, graphiteThin films prepared by eBeam evaporation of powdered source material have been reported. RF Sputter deposition is widely reported
WTe39.49
WO314737.16980eBeam (good)WThin films are most commonly prepared using WO3 powder source material
sublimes
U113219.07113213271582eBeam (good)W, Mo, graphiteDepleted uranium thin films oxidize easily even in low partial pressure of O2
UC2226011.282100
UO2217610.9eBeam (fair)WStoichiometric thin films produced by reactive evaporation of depleted uranium in O2 partial pressure have been reported
UF4~1000300Thin films fabricated by sputter deposition of depleted uranium by F– ions has been reported
U3O8Decomposes8.3Thin films produced by reactive sputter deposition of depleted uranium targets in O2 have been reported.
UP28.571200
U2S31400
V18905.96116213321547eBeam (Xlnt)W, graphite, TaWets Mo. eBeam evaporation is preferred
VB224005.1
VC28105.77~1800
VO219674.34~575eBeam (poor)W, graphiteDifficult to maintain stoichiometry by eBeam evaporation, sputter deposition is preferred
sublimes
VN23206.13
V2O56903.36~500eBeam (good)W, graphiteThin films prepared from powdered source material are nearly stoichiometric. Post process annealing at 280° in O2 restores full stoichiometry
VSi217004.42
Yb8246.98520590690eBeam (good)Al2O3, W, TaStore Yb evaporation source material in N2 desiccator to mitigate oxidation
sublimes
YbF311578.17~800eBeam (fair)Ta, Mo, WPreheat slowly and evaporate at
≤ 10Å/sec to mitigate dissociation
Yb2O323469.17~1500eBeam (fair)Al2O3, W, TaThin films produced by reactive evaporation in 8 x 10-5 torr O have
2
sublimesbeen reported.
Y15094.488309731157eBeam (Xlnt)W, Al2O3Substrate heating at 300°C improves adhesion and film smoothness
Y3Al5O121990eBeam (good)W, Al2O3Films prepared from powdered source material, typically with dopants. YAG films post deposition annealed at 1100°C in vacuum improves crystallinity
YF313874.01eBeam (good)W, Ta, Mo, Al2O3eBeam evaporation at a rate of
≤ 10Å/sec and substrate temperature of 200°C produces crystalline films with good adhesion
Y2O326804.84~2000eBeam (good)graphite, WeBeam evaporated films can be oxygen deficient, post deposition annealing
in 10-3 torr O at 525°C results in
2
sublimesstoichiometric films.
Zn4197.140.514127177250eBeam (Xlnt)W, Al2O3, quartz, graphiteEvaporates well under a wide range of conditions
Zn3Sb25466.3
ZnBr23944.22~300
ZnF2874.84~800eBeam (fair)quartz, WThin films prepared by eBeam evaporation of powdered source material have been reported. Substrate heating at 400°C improved crystallinity
Zn3N26.22Reactive sputter deposition in N2 has been reported
ZnO19755.61~1800eBeam (fair)quartz, WQuality thin films fabricated using eBeam evaporation at a rate of 8Å/sec and a substrate temperature of 300°C has been reported
ZnSe15265.42660eBeam (fair)W, Ta, Mo,Deposition rate of ≤ 5 Å/sec. Thin films are polycrystalline and a substrate temperature of 300°C improves adhesion and size of crystallites
quartz
ZnS18304.09~800eBeam (good)W, Ta, Mo,Thin films produced by eBeam evaporation display a preferred (111) orientation and best optical properties result from a 400°C substrate temperature
sublimesquartz
ZnTe12386.34~600eBeam (fair)W, Ta, Mo,Stoichiometric thin films produced by eBeam evaporation have good
quartzcrystallinity with a substrate temperature of 230°C. Optical properties are thickness dependent
ZrSiO425504.56
Zr18526.4147717021987eBeam (Xlnt)W, quartzAlloys with W. Thin films oxidize readily
ZrB230406.08eBeam (good)W, quartzStoichiometric films prepared by
co-evaporation of Zr and B have been reported
ZrC35406.73~2500eBeam (poor)graphiteQuality thin films of ZrC using pulsed laser deposition have been reported
ZrN29807.09Thin films of ZrN prepared by N2 ion assisted evaporation of Zr have been reported
ZrO227005.49~220eBeam (good)W, graphiteReactive evaporation in 10-3 torr O
2
produce as deposited stoichiometric
films. For eBeam evaporated films, post deposition annealing in O2 restores stoichiometry
ZrSi217004.88eBeam evaporated Zr on Si substrates forms ZrSi2 following post deposition thermal annealing at 600°C

Advantages of Evaporation Coating

High Purity of Thin Film

Evaporation coating is carried out in a high vacuum environment, and the vacuum degree can usually reach 10⁻6Pa or even higher. It greatly reduces the chances of impurities such as oxygen, nitrogen, and water vapor in the air reacting with evaporated atoms or molecules, and also avoids the mixing of impurity particles into the film.

Good Film Uniformity

In evaporation coating, the shape and position of the evaporation source and the movement of the substrate (such as substrate rotation) are reasonably designed to make the evaporated atoms or molecules deposited evenly on the substrate surface. Effectively eliminate the radial difference in film thickness.

Low Cost

Compared with some other thin film preparation technologies (such as chemical vapor deposition, sputtering coating, etc.), the structure of evaporation coating equipment is relatively simple. The cost of manufacturing thin films is relatively low.

Fast Deposition Rate

Evaporation coating can achieve a high deposition rate, which can generally reach a few nanometers to tens of nanometers per second. This means improving efficiency, reducing costs, and reducing the risk of substrate contamination.

Wide Material Adaptability

Evaporation coating technology is applicable to a variety of materials, including metals, non-metals, compounds and some organic materials. This enables evaporation coating technology to meet the diverse needs of thin film materials in different fields.

Strong Bonding Force

By controlling evaporation parameters (such as substrate temperature and evaporation rate), the bonding force between the film and the substrate can be effectively adjusted. Enable atoms to be more closely bonded to the substrate surface.

Disadvantages of Evaporation Coating

Although evaporation coating has many advantages, it also has some inherent disadvantages and limitations in practical applications. These disadvantages limit its application in certain fields to a certain extent.

High Purity of Thin Film

Evaporation coating is carried out in a high vacuum environment, and the vacuum degree can usually reach 10⁻6Pa or even higher. It greatly reduces the chances of impurities such as oxygen, nitrogen, and water vapor in the air reacting with evaporated atoms or molecules, and also avoids the mixing of impurity particles into the film.

Incompatible With High Melting Point Materials

For high melting point materials (such as tungsten, molybdenum, silicon carbide, etc.), the evaporation temperature is extremely high, usually reaching several thousand degrees Celsius. It is difficult to heat these materials to the evaporation temperature.

Large Film Stress

The growth of thin films is affected by many factors (such as the difference in thermal expansion coefficient between the substrate and the film, too fast atomic deposition rate, etc.), resulting in large stress inside the film.

Compound materials are easy to decompose

For organic compound materials, their molecular structure is relatively complex. During heating and evaporation, the chemical bonds between molecules may break, causing the decomposition of organic materials.

Application of Evaporation Coating

Due to its unique advantages, evaporation coating technology has been widely used in many fields and has provided important technical support for the development of various industries.

Sensor

The sensitive elements of many sensors (such as temperature sensors, gas sensors, pressure sensors, etc.) require coating technology support. For example, in gas sensors, metal oxide films (such as zinc oxide, tin oxide, etc.) are prepared by evaporation coating. This has sensitive electrical property changes to specific gases, and gas detection can be achieved by detecting its resistance changes. Evaporation coating technology can accurately control the thickness and composition of the film to ensure the sensitivity and stability of the sensor.

Sensor

Optics

Evaporation coating technology is widely used in the coating of optical lenses, including anti-reflection film, high reflective film, filter, etc. In storage media such as optical discs (such as CD, DVD, Blu-ray disc), evaporation coating is used to prepare reflective layer and recording layer. The core component of solar cells is semiconductor film that absorbs sunlight and converts it into electrical energy. Evaporation coating technology supports the preparation of various films in solar cells, such as transparent conductive film (ITO film), electrode film, absorption layer film, etc.

Optical Field

Medical

Some medical devices (such as scalpels, syringes, artificial joints, etc.) require surface treatment to improve their performance and biocompatibility. Evaporation coating technology supports the deposition of biocompatible films on the surface of medical devices, such as titanium films, titanium nitride films, etc. Improve the wear resistance, corrosion resistance and biocompatibility of the device.

Medical

Conclusion

As an important physical vapor deposition technology, evaporation coating technology has developed for more than a hundred years and has formed a relatively complete theoretical system and diversified process methods. From the early simple resistance evaporation to today’s advanced technologies such as laser evaporation and electron beam evaporation, evaporation coating is expanding its application boundaries in continuous innovation. Its core principle is to evaporate the coating material into gaseous atoms or molecules through a specific heating method in a high vacuum environment. These particles are transmitted in a vacuum and deposited on the substrate surface, and form a thin film through adsorption, diffusion, nucleation and growth.

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